3 /Ga3 雙摻雜的石榴石型Yb3-xGdxAl5-xGaxO12固溶體陶瓷材料 (x=0.0,0.1,0.2,0.3,0.4,0.5;YGAGO)。結(jié)果表明:Gd3 /Ga3 共摻雜的YGAGO保持了石榴石相結(jié)構(gòu);隨著Gd3 /Ga3 摻雜量的增加,固溶體樣品的衍射峰位整體向低角度偏移;SEM形貌表明Yb3Al5O12材料的微觀形貌由納米級(jí)晶粒和高密度晶界構(gòu)成;大離子Gd3 與Ga3 分別對(duì)Yb3Al5O12晶體結(jié)構(gòu)中Yb3 與Al3 晶格位的取代,不僅因引入的點(diǎn)缺陷明顯降低了材料的熱導(dǎo)率,同時(shí)還造成石榴石型Yb3Al5O12晶體結(jié)構(gòu)的松弛,利于熱膨脹系數(shù)的提高。隨著Gd3 /Ga3 摻雜量的增加,晶體中點(diǎn)缺陷濃度不斷升高,聲子平均自由程不斷減小,使得YGAGO的熱導(dǎo)率在x=0.5時(shí)達(dá)到最低值(λ=1.67W/m.K,T=1273K),熱膨脹系數(shù)達(dá)到最高值(ɑl=11.71×10-6 K-1,T=1273K)。"/>
內(nèi)蒙古科技大學(xué)數(shù)理生學(xué)院,內(nèi)蒙古科技大學(xué)數(shù)理生學(xué)院
內(nèi)蒙古自然科學(xué)基金資助
School of Mathematics,Physics and Biological Engineering,Inner Mongolia University of Science and Technology,School of Mathematics,Physics and Biological Engineering,Inner Mongolia University of Science and Technology
李劍生,劉艷麗. Gd3 /Ga3 共摻雜石榴石型Yb3Al5O12材料的制備及熱物理性能[J].稀有金屬材料與工程,2017,46(3):802~806.[Li Jiansheng, Liu Yanli. Preparation and Thermo-Physical Properties of Gd3 /Ga3 Co-doped Garnet-type Yb3Al5O12[J]. Rare Metal Materials and Engineering,2017,46(3):802~806.]
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