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La0.82Te0.18MnO3薄膜的龐磁電阻效應及光誘導特性
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TQ174

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國家自然科學基金(50331040,60171034)和西北工業(yè)大學博士論文創(chuàng)新基金(CX200615)


CMR Effect and the Photo-Induced Properties in La0.52Te0.18MnO3 Thin Film
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    摘要:

    用脈沖激光沉積(PLD)法在LaAlO3單晶襯底上制備了VIA族非金屬元素Te摻雜的La0.82Te0.18MnO3(LTMO)薄膜。X射線衍射分析表明,薄膜具有鈣鈦礦贗立方結構,且沿(012)方向擇優(yōu)生長;電阻-溫度關系顯示,該材料存在金屬-絕緣體轉變特性和龐磁電阻(CMR)效應;在0.7T的磁場作用下,薄膜的磁電阻最大值為30.6%,對應的溫度在263K。而室溫(303K)磁電阻值為4.8%;擬合分析表明,薄膜在低溫區(qū)是單磁子散射,在高溫區(qū)滿足小極化子輸運模型。在波長為532nm的綠激光作用下,在253K,光致電阻變化率達到最大值33.6%;分析認為這可能是由于光激發(fā)會改變材料中的磁有序,減弱雙交換作用,進而改變電子的輸運性質。

    Abstract:

    Using pulsed laser deposition method, the La0.82Te0.18MnO3 thin film was prepared on LaAlO3 (012) single crystal substrate. The structure of the film studied by X-ray diffractometry shows that the film has perovskite pseudocubic structure, and is of preferential orientation (012). The R-T curves show the metal-insulator transition (MIT) and CMR effect. And the TMI are 283 K and 303 K for 0 T and 0.7 T, respectively, and they are both near room temperature. The maximum MR is 30.6% at 0.7 T. Correspondingly, the peak temperature at the maximum MR is 263 K. This shows that the films display CMR effect in the mental region. Moreover, the magnetoresistance ratio at the room temperature (303 K) is 4.8% at 0.7 T. The results show that the data satisfy R=P1+P2T2+P3T4.5 for TTMI, it is satisfied with small polaron model. The effect of the continuous wave laser (532 nm, 40 mW) on the film was also investigated. Below TMI, the resistance increased under photo inducing. Above TMI there was a decrease of the resistance. The maximum photoinduced resistance change is 33.6%. This is attributed to the change of the magnetic order in the film because of photoinducing, which might reduce the double exchange, and change electronic transport.

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高國棉 陳長樂 王建元 韓立安 王永倉 宋宙模. La0.82Te0.18MnO3薄膜的龐磁電阻效應及光誘導特性[J].稀有金屬材料與工程,2007,36(4):644~647.[Gao Guomian, Chen Changle, Wang Jianyuan, Han Lian, Wang Yongcang, Song Zhoumo. CMR Effect and the Photo-Induced Properties in La0.52Te0.18MnO3 Thin Film[J]. Rare Metal Materials and Engineering,2007,36(4):644~647.]
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  • 最后修改日期:2006-07-18
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